Numerous children she visited were victims of the terrorist attack that followed her Manchester concert on May 22, in which 22 people were killed and 59 injured.
Sunday's One Love Manchester concert has become the biggest TV show of the year so far - attracting a peak audience of more than 14 million viewers in the United Kingdom, with worldwide ratings expected to top 100 million.
"I think that the kind of love, the unity that you're displaying is the medicine that the world really needs right now", the 23-year-old told the 50,000-person crowd.
After the One Love Manchester gig over the weekend, the team were joined backstage by artists from Manchester Ink to get inked with a symbol of the city.
The superstar debuted her new song titled "Inspired" during a recent performance on the Today show, revealing that she wrote it about her dad, country singer Billy Ray Cyrus.
Chris Martin and Jonny Buckland of Coldplay performed it delicately, dedicating it to Grande herself, and this time, Manchester sung it even louder.
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Grande invited the members of a local high school choir (many of whom were present at her first show) to perform with her on stage. "We must not be afraid and in tribute to all those affected here and around the world, we will bring our voices together and sing loudly". By re-releasing one of her biggest hits, the songstress is making it clear that she has nothing but love for everyone involved.
The concert, held by Ariana Grande, happened last night.
Grande paid tribute to her fans, including Olivia Campbell, 15, at her One Love concert at the Old Trafford Cricket Ground on Sunday evening as concert goers proudly wore clothes emblazoned with the slogan, "We stand together". Aside from helping raise $13 million for the We Love Manchester Emergency Fund that will help those who suffered from the attack, Bieber offered some spirit-filled words to those viewing his performances of "Love Yourself" and "Cold Water". "We love you so much, to the families we love you so much".
Other performers will include Pharrell Williams, Usher, the Black Eyed Peas, Robbie Williams and Niall Horan.
'I love you guys so much.
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